2009, English, Article edition: Realization of time-resolved two-vacuum-ultraviolet-photon ionization Peralta Conde, A.; Kruse, J.; Faucher, O.; ...

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Physical Description
  • text
Published
  • HAL - CCSD
  • 2009
Language
  • English

Edition details

Title
  • Realization of time-resolved two-vacuum-ultraviolet-photon ionization
Author
  • Peralta Conde, A.
  • Kruse, J.
  • Faucher, O.
  • Tzallas, P.
  • Benis, E. P.
  • Charalambidis, D.
Published
  • HAL - CCSD
  • 2009
Physical Description
  • text
Subjects
Notes
  • Ultrafast dynamics of excited molecules is studied through time-resolved two-vacuum-ultraviolet (vuv)- photon ionization using a nonlinear volume autocorrelator unit. The two-vuv-photon process is induced by the intense fifth harmonic radiation of a femtosecond Ti:sapphire laser. In a proof-of-principle experiment, ultrafast dynamics of excited ethylene and oxygen molecules are investigated. Molecular decay times are deduced by comparing the experimental data with the results of a numerical model that accounts for the spatial and temporal characteristics of the harmonic field. The present experiments pave a convenient way for time domain investigations in the vuv-xuv spectral region in all states of matter at few femtosecond to subfemtosecond temporal scales.
  • HAL:hal-00402819, version 1
  • HAL:http:/​/​hal.archives-ouvertes.fr/​hal-00402819/​en/​
  • DOI:10.1103/​PhysRevA.79.061405
Language
  • English
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